Catalan leader Carles Puigdemont says the region has won the right to statehood following Sunday's contentious referendum which was marred by violence.
He said the door had been opened to a unilateral declaration of independence.
Catalan officials later said 90% of those who voted backed independence. The turnout was 42.3%.
Hundreds of people were injured as Spanish police used force to try to block voting.
The Spanish government had pledged to stop a referendum that was declared illegal by the country's constitutional court.
Police officers prevented some people from voting, and seized ballot papers and boxes at polling stations.
"With this day of hope and suffering, the citizens of Catalonia have won the right to an independent state in the form a republic," Mr Puigdemont said in a televised address flanked by other senior Catalan leaders.
"My government, in the next few days will send the results of today's vote to the Catalan parliament, where the sovereignty of our people lies, so that it can act in accordance with the law of the referendum."
He said the European Union could no longer "continue to look the other way".
The Catalan government said more than 800 people had been injured in clashes across the region. Those figures included people who had suffered relatively minor complaints such as anxiety attacks.
In another development, more than 40 trade unions and Catalan associations called a region-wide strike on Tuesday due to "the grave violation of rights and freedoms".
Earlier, as voting ended, Spanish Prime Minister Mariano Rajoy said Catalans had been fooled into taking part in an illegal vote. He called it a "mockery" of democracy.
Large crowds of independence supporters gathered in the centre of the regional capital Barcelona on Sunday evening, waving flags and singing the Catalan anthem.
Source: BBC
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